| Hiroki Ago | Last modified date:2013.5.24 |
Associate Professor /
Department of Integrated Materials
Institute for Materials Chemistry and Engineering
Institute for Materials Chemistry and Engineering
Graduate School
E-Mail
Homepage
[URL]
Research on growth and electronic applications of graphene and carbon nanotubes .
Fax
092-583-7817
Academic Degree
Doctor of Engineering
Field of Specialization
Nanotechnology, Physical Chemistry, Molecular Engineering, Material Science
Outline Activities
Research activities:
Carbon nanotubes are one of attractive nano-materials due to their unique electronic structure. The following research subjects are in progess.
[1] Growth, mechanism, and processing of high-quality graphene
[2] Electrical and/or chemical applications of graphene and nanotubes
[3] Developpment of new two dimensional nanosheets
[4] Highly-controlled synthesis and large-scale production of single-walled carbon nanotubes
Education activities:
Teaching in classes both in the undergraduate and graduate schools.
Carbon nanotubes are one of attractive nano-materials due to their unique electronic structure. The following research subjects are in progess.
[1] Growth, mechanism, and processing of high-quality graphene
[2] Electrical and/or chemical applications of graphene and nanotubes
[3] Developpment of new two dimensional nanosheets
[4] Highly-controlled synthesis and large-scale production of single-walled carbon nanotubes
Education activities:
Teaching in classes both in the undergraduate and graduate schools.
Research
Research Interests
- Synthesis of novel carbon materials
keyword : nanocarbon
2012.04. - Growth and Development of new two-dimensional materials
keyword : two-dimensional materials
2012.04. - Electronic and optical properties of graphene and development of electronic applications
keyword : graphene, CVD, physical properties devices
2011.04. - Development of processing methods of graphene
keyword : graphene, CVD, processing
2010.04. - Catalytic growth of graphene films and understanding the growth mechanism
keyword : graphene, cystal growth, CVD
2011.04. - Development of highly controlled synthesis of single-walled carbon nanotubes - chirality/electronic structure control-
keyword : carbon nanotube, chirality, semiconductor
2007.10. - Epitaxially aligned growth and high-density growth of single-walled carbon nanotubes
keyword : single-walled carbon nanotubes, horizontally-aligned growth
2004.10. - Basic research for electronic applications of single-walled carbon nanotubes
keyword : carbon nanotubes, transistors
2005.04.
- Synthesis and Control of Graphene for Carbon Electronics
- Synthesis and Control of Graphene for Carbon Electronics
- Epitaxial growth of single-walled carbon nanotubes on crystalline surfaces.
- Fabrication of ordered carbon nanotube network and application to next-generation semiconductor devices.
Books
| 1. | Carbon Nanotubes - Challenge to nanodevices - Chap. 11; Workfunction and integrated devices with semiconductors, H. Ago K. Tanaka ed.. |
| 2. | H. Ago and T. Yamabe,The Science and Technology of Carbon Nanotubes,Elsevier Science, Oxford, UK,Frontiers in Carbon Nanotubes and Beyond, Chap. 14, p.163-183,1999.01. |
Papers
| 1. | Y. Ogawa, B. Hu, C. M. Orofeo, M. Tsuji, K. Ikeda, S. Mizuno, H. Hibino, H. Ago,Domain structure and boundary in single-layer graphene grown on Cu (111) and Cu (100) films,J. Phys. Chem. Lett.,Vol.3,No.2,pp.219-226,2012.01. |
| 2. | B. Hu, H. Ago,* Y. Ito, K. Kawahara, M. Tsuji, E. Magome, K. Sumitani, N. Mizuta, K. Ikeda, S. Mizuno,Epitaxial growth of large-area single-layer graphene over Cu(111)/sapphire by atmospheric pressure CVD,Carbon,Vol.50,No.1,pp.57-65,2012.01. |
| 3. | H. Ago, T. Ayagaki, Y. Ogawa, M. Tsuji,Ultra-high vacuum-assisted control of metal nanoparticles for horizontally-aligned single-walled carbon nanotubes with extraordinary uniform diameters,J. Phys. Chem. C,Vol.115,No.27,pp.13247-13253,2011.07. |
| 4. | C. M. Orofeo, H. Ago, B. Hu, M. Tsuji,Synthesis of large-area, homogeneous, single layer graphene by annealing amorphous carbon on Co and Ni,Nano Res.,Vol.4,No.6,pp.531-540,2011.06. |
| 5. | H. Ago, Y. Ito, N. Mizuta, K. Yoshida, B. Hu, C. M. Orofeo, M. Tsuji, K. Ikeda, S. Mizuno,Epitaxial chemical vapor deposition growth of single-layer graphene over cobalt film crystallized on sapphire,ACS Nano,Vol.4,No.12,pp.7407-7414,2010.12. |
| 6. | H. Ago, T. Nishi, K. Imamoto, N. Ishigami, M. Tsuji, T. Ikuta, K. Takahashi ,Orthogonal growth of horizontally-aligned single-walled carbon nanotube arrays,J. Phys. Chem. C,Vol.114,No.30,pp.12925-12930,2010.08. |
| 7. | H. Ago, I. Tanaka, M. Tsuji, K. Ikeda,Patterned growth of graphene over epitaxial catalyst,Small,Vol.6,No.11,pp.1226-1233,2010.06. |
| 8. | H. Ago, K. Imamoto, T. Nishi, M. Tsuji, T. Ikuta, and K. Takahashi,Direct growth of bent carbon nanotubes on surface engineered sapphire,J. Phys. Chem. C,113(30), 13121-13124.,2009.07. |
| 9. | N. Yoshihara, H. Ago, M. Tsuji, T. Ikuta, and K. Takahashi,Horizontally aligned growth of single-walled carbon nanotubes on surface modified silicon wafer,J. Phys. Chem. C,113(19), 8030-8034,2009.05. |
| 10. | C. M. Orofeo, H. Ago,* N. Yoshihara, and M. Tsuji,Top-down approach to align single-walled carbon nanotubes on silicon substrate,Appl. Phys. Lett.,94(5), 053113-1-3,2009.02. |
| 11. | N. Ishigami, H. Ago, T. Nishi, K. Ikeda, M. Tsuji, T. Ikuta, and K. Takahashi ,Unidirectional growth of single-walled carbon nanotubes,J. Am. Chem. Soc. ,130(51), 17264-17265,2008.12. |
| 12. | N. Ishigami, H. Ago, K. Imamoto, M. Tsuji, K. Iakoubovskii, and N. Minami,Crystal plane dependent growth of aligned single-walled carbon nanotubes on sapphire,J. Am. Chem. Soc.,130(30), 9918-9924 (2008). ,2008.07. |
| 13. | H. Ago, N. Ishigami, N. Yoshihara, K. Imamoto, K. Ikeda, M. Tsuji, T. Ikuta, and K. Takahashi,Visualization of horizontally-aligned single-walled carbon nanotube growth with 13C/12C isotopes,J. Phys. Chem. C,J. Phys. Chem. C (Letter), 112(6), 1735-1738 (2008.2). selected as cover,2008.02. |
| 14. | N. Ishigami, H. Ago, Y. Motoyama, M. Takasaki, M. Shinagawa, K. Takahashi, K. Takahashi, and M. Tsuji,Microreactor utilizing a vertically-aligned carbon nanotube array grown inside the channels,Chem. Commun.,1626-1628,2007.03. |
| 15. | H. Ago, K. Imamoto, N. Ishigami, R. Ohdo, K. Ikeda, and M. Tsuji,Competition and cooperation between lattice-oriented growth and step-templated growth on aligned carbon nanotubes on sapphire,Appl. Phys. Lett.,90(12), 123112-1-3,2007.03. |
| 16. | H. Ago, N. Uehara, N. Yoshihara, M. Tsuji, M. Yumura, N. Tomonaga, and T. Setoguchi,Gas analysis of CVD process for high yield growth of carbon nanotubes over metal-supported catalysts,Carbon,44(14), 2912-2918 ,2006.11. |
| 17. | H. Ago, K. Nakamua, K. Ikeda, N. Uehara, N. Ishigami, and M. Tsuji,Aligned growth of isolated single-walled carbon nanotubes programmed by atomic arrangement of substrate surface,Chem. Phys. Lett.,Vol.408,No.4-6,408(4-6), 433-438 (2005).,2005.06. |
| 18. | H. Ago, S. Imamura, T. Okazaki, T. Saito, M. Yumura, and M. Tsuji,CVD growth of single-walled carbon nanotubes with a narrow diameter distribution and their optical properties",J. Phys. Chem. B,Vol.109,No.20,109(20), 10035-10041 (2005).,2005.05. |
| 19. | H. Ago, S. Ohshima, K. Tsukagoshi, M. Tsuji, and M. Yumura,Formation mechanism of carbon nanotubes in the gas-phase synthesis from colloidal solutions of nanoparticles,Curr. Appl. Phys.,Vol.5,No.2,5(2), 128-132 (2005).,2005.02. |
| 20. | H. Ago, K. Nakamura, N. Uehara, and M. Tsuji,Roles of meal-support interaction in growth of single- and double-walled carbon nanotubes studied with diameter-controlled iron particles supported on MgO,J. Phys. Chem. B,108 (49), 18908-18915 (2004).,2004.12. |
| 21. | H. Ago, K. Nakamura, S. Imamura, and M. Tsuji,Growth of double-wall carbon nanotube with diameter-controlled iron oxide nanoparticles supported on MgO,Chemical Physics Letters,Vol.391,No.4-6,391(4-6), 308-313 (2004).,2004.06. |
| 22. | Y. Zhang, H. Ago, J. Liu, M. Yumura, K. Uchida S. Ohshima, S. Iijima, J. Zhu, X. Zhang,The synthesis of In, In2O3 nanowires and In2O3 nanoparticles with shape-controlled,Journal of Crystal Growth,264, 363-368 (2004).,2004.04. |
| 23. | H. Ago, J. Qi, K. Tsukagoshi, K. Murata, S. Ohshima, Y. Aoyagi, and M. Yumura,Catalytic growth of carbon nanotubes and their patterning based on ink-jet and lithographic techniques,Journal of Electroanalytical Chemistry,559, 25-30 (2003).,2003.11. |
| 24. | H. Ago, K. Murata, M. Yumura, J. Yotani, and S. Uemura,Ink-Jet Printing of Nanoparticle Catalyst for Site-Selective Carbon Nanotube Growth,Applied Physics Letters,82(5), 811-813 (2003).,2003.02. |
| 25. | T. Kimura, H. Ago, M. Tobita, S. Ohshima, M. Kyotani, and M. Yumura,Polymer Composites of Carbon Nanotubes Aligned by a Magnetic Field,Advanced Materials,14(19), 1380-1383 (2002).,2002.10. |
| 26. | H. Ago, S. Ohshima, K. Uchida, T. Komatsu, and M. Yumura,Carbon nanotube synthesis using colloidal solution of metal nanoparticles,Physica B,323(1-4), 306-307 (2002).,2002.10. |
| 27. | H. Ago, S. Ohshima, K. Uchida, and M. Yumura,Gas-phase synthesis of single-wall carbon nanotubes from colloidal solution of metal nanoparticles,The Journal of Physical Chemistry B,105(43), 10453-10456 (2001).,2001.11. |
| 28. | H. Ago, T. Komatsu, S. Ohshima, Y. Kuriki, and M. Yumura,Dispersion of metal nanoparticles for aligned multiwall carbon nanotube arrays,Applied Physics Letters,77(1), 79-81 (2000).,2000.07. |
| 29. | H. Ago, M. S. P. Shaffer, D.S. Ginger, A. H. Windle, and R. H. Friend,Electronic interaction bewteen photo-excited poly(p-phenylene vinylene) and carbon nanotubes,Physical Review B,61(3), 2286-2290 (2000).,2000.01. |
| 30. | H. Ago, K. Petritsch, M. S. P. Shaffer, A. H. Windle, and R. H. Friend,Composites of carbon nanotubes and conjugated polymers for photovoltaic devices,Advanced Materials,11(15), 1281-1285 (1999).,1999.10. |
| 31. | K. Tsukagoshi, B. W. Alphenaar, and H. Ago,Coherent transport of electron spin in a ferromagnetically contacted carbon nanotube,Nature,401, 572-574 (1999).,1999.10. |
| 32. | H. Ago, Th. Kugler, F. Cacialli, W. R. Salaneck, M. S. P. Shaffer, A. H. Windle, and R. H. Friend,Work functions and surface functional groups of multiwall carbon nanotubes,The Journal of Physical Chemistry B,103(38), 8116-8121 (1999).,1999.09. |
| 33. | H. Ago, M. Kato, K. Yahara, K. Yoshizawa, K. Tanaka, and T. Yamabe,Ab initio study on interaction and stability of lithium-doped amorphous carbons,Journal of the Electrochemical Society,146(4), 1262-1269 (1999).,1999.04. |
| 34. | H. Ago, K. Tanaka, T. Yamabe, K. Takegoshi, T. Terao, S. Yata, Y. Hato, and N. Ando,7Li NMR study of Li-doped polyacenic semiconductor (PAS) materials,Synthetic Metals,89, 141 (1997).,1997.08. |
| 35. | H. Ago, K. Tanaka, T. Yamabe, T. Miyoshi, K. Takegoshi, T. Terao, S. Yata, Y. Hato, and N. Ando,Structural analysis of polyacenic semiconductor (PAS) materials with 129Xe NMR measurements,Carbon,35, 1781-1787 (1997).,1997.12. |
| 36. | H. Ago, T. Kuga, T. Yamabe, K. Tanaka, A. Kunai, and M. Ishikawa,Electronic properties of p-type doped copolymers consisting of oligothienylene and disilanylene units,Chemistry of Materials,9, 1159-1165 (1997).,1997.05. |
| 37. | H. Ago, K. Nagata, K. Yoshizawa, K. Tanaka, and T. Yamabe,Theoretical study of Li-doped polycyclic aromatic hydrocarbons,Bulletin of the Chemical Society of Japan,70, 1717-1726 (1997).,1997.07. |
| 38. | H. Ago, T. Kuga, T. Yamabe, K. Tanaka, S. Yata, Y. Hato, and N. Ando,ESR study of alkali-doped polyacenic semiconductor (PAS) materials prepared by thermal decomposition of azides,Carbon,35, 651-656 (1997).,1997.12. |
Presentations
Membership in Academic Society
| 1. | Surface atomic arrangement-programmed growth of horizontally-aligned SWNTs on sapphire. |
| 2. | Aligned growth of single-walled carbon nanotubes programmed by single crystal surface. |
| 3. | Aligned growth of single-walled carbon annotubes and their characterization. |
- The Fullerenes, Nanotubes, and Graphene Research Society
- The Japan Society of Applied Physics
- Chemical Society of Japan
- Iijima award
- Tsukuba prize (industrial part)
Educational
The fact that no permission it reprints contents of this data base is prohibitted.

