Kyushu University Academic Staff Educational and Research Activities Database
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Tomohiro Shiraki Last modified date:2019.06.14

Associate Professor / Molecular Information Chemistry
Department of Applied Chemistry
Faculty of Engineering


Graduate School
Undergraduate School
Other Organization


E-Mail
Homepage
http://www.chem.kyushu-u.ac.jp/~fifth/en
Phone
092-802-2841
Fax
092-802-2840
Academic Degree
Ph.D.
Country of degree conferring institution (Overseas)
No
Field of Specialization
Nanocarbon Chemistry, Supramolecular Chemistry, Polymer Chemistry, Mechanochemistry
Total Priod of education and research career in the foreign country
02years00months
Outline Activities
[Research]
Nanomaterial fabrication through supramolecular chemistry techniques. Functionalization of carbon nanomaterials based on molecular design approaches.

[Education]
Experimental lectures for undergraduate students
Research guidance for group members of Doctor, Master, and Undergraduate students
Research
Research Interests
  • Synthesis and characterization of new porous materials
    keyword : Supramolecular chemistry, Polymer Chemistry
    2015.04~2020.03.
  • Functionalization of nanocarbon materials based on molecular designs
    keyword : Supramolecular chemistry, Nanocarbon, Polymer Chemistry
    2015.04~2020.03.
  • Nanocarbon chemistry through supramolecular approaches
    keyword : Supramolecular chemistry, Nanocarbon
    2014.04~2020.03.
Academic Activities
Books
1. Munenori Numata, Kouta Sugikawa, Shuichi Haraguchi, Tomohiro Shiraki, Shun-ichi Tamaru, Shingo Tamesue, Seiji Shinkai, Beta-Glucans: Applications, Effects and Research:Chapter 2 Supramolecular Wrapping by Beta-(1¨3)-D-Glucans toward Polysaccharide-Based Functional Materials , Nova Science Publishers , ebook ISBN:978-1-53610-655-8, 2017.02.
Papers
1. Tomohiro Shiraki, Boda Yu, Tomonari Shiraishi, Tamehito Shiga, Tsuyohiko Fujigaya, Meta-linkage design of bis-aryldiazonium modifiers for wavelength tuning of near infrared photoluminescence from locally functionalized single-walled carbon nanotubes, Chemistry Letters, in press, 2019.04.
2. Tomohiro Shiraki, Yoshiaki Niidome, Fumiyuki Toshimitsu, Tomonari Shiraishi, Tamehito Shiga, Boda Yu, Tsuyohiko Fujigaya, Solvatochromism of near infrared photoluminescence from doped sites of locally functionalized single-walled carbon nanotubes, Chemical Communications, DOI: 10.1039/C9CC00829B, 55, 3662-3665 , 2019.03.
3. Edyta Turek, Tomohiro Shiraki, Tomonari Shiraishi, Tamehito Shiga, Tsuyohiko Fujigaya, Dawid Janas, Single-step isolation of carbon nanotubes with narrow-band light emission characteristics, Scientific Reports, DOI: 10.1038/s41598-018-37675-4, 9, 535, 2019.01.
4. Tomohiro Shiraki, Tamehito Shiga, Tomonari Shiraishi, Hisashi Onitsuka, Naotoshi Nakashima, Tsuyohiko Fujigaya, Multistep Wavelength Switching of Near‐infrared Photoluminescence Driven by Chemical Reactions at Local Doped Sites of Single‐walled Carbon Nanotubes, Chemistry - A European Journal, DOI: 10.1002/chem.201805342, 24, 19162-19165, 2018.12.
5. Keita Ozono, Masashi Fukuzawa, Fumiyuki Toshimitsu, Tomohiro Shiraki, Tsuyohiko Fujigaya, Naotoshi Nakashima, Chiral Selective Chemical Reaction of Flavin-derivative-wrapped Semiconducting Single-walled Carbon Nanotubes Based on a Specific Recognition, Bulletin of the Chemical Society of Japan, 10.1246/bcsj.20180206, 91, 1646-1651, 2018.09.
6. Hisashi Onitsuka, Tsuyohiko Fujigaya, Naotoshi Nakashima, Tomohiro Shiraki, Control of the near infrared photoluminescence of locally functionalized single-walled carbon nanotubes via doping by azacrown-ether modification, Chemistry - A European Journal, 10.1002/chem.201800904, 24, 9393-9398, 2018.05.
7. Tomohiro SHIRAKI, Shunsuke UCHIMURA, Tomonari SHIRAISHI, Hisashi ONITSUKA, Naotoshi NAKASHIMA, Near Infrared Photoluminescence Modulation by Defect Site Design Using Aryl Isomers in Locally Functionalized Single-walled Carbon Nanotubes, Chemical Communications, 10.1039/C7CC06663E, 53, 12544-12547, 2017.10.
8. Tomonari SHIRAISHI, Tomohiro SHIRAKI, Naotoshi NAKASHIMA, Substituent Effects on the Redox States of Locally Functionalized Single-Walled Carbon Nanotubes Revealed by in situ Photoluminescence Spectroelectrochemistry, Nanoscale, 10.1039/C7NR05480G, 9, 16900-16907, 2017.10.
9. Gayoung Kim, Jun Yang, Naotoshi Nakashima, Tomohiro Shiraki, Highly microporous nitrogen-doped carbon synthesized from azine-linked covalent organic framework and its supercapacitor function, Chemistry - A European Journal, 10.1002/chem.201702805, 23, 69, 17504-17510, accepted, Selected as Hot paper and inside cover, 2017.09.
10. Tomohiro SHIRAKI, Hisashi Onitsuka, Tomonari Shiraishi, Naotoshi NAKASHIMA, Near Infrared Photoluminescence Modulation of Single-Walled Carbon Nanotubes Based on a Molecular Recognition Approach, Chemical Communications, 10.1039/C6CC07287A, 52, 12972-12975, 2016.10.
11. Naotoshi NAKASHIMA, Tomohiro SHIRAKI, Specific Molecular Interaction and Recognition at Single-walled Carbon Nanotube Surfaces, Langmuir, 10.1021/acs.langmuir.6b02023, 32, 12323-12331, 2016.07.
12. Tomohiro SHIRAKI, Tomonari Shiraishi, JUHASZ GERGELY MIKLOS, Naotoshi NAKASHIMA, Emergence of new red-shifted carbon nanotube photoluminescence based on proximal doped-site design, Scientific Reports, 10.1038/srep28393, 6, 28393, 2016.06.
13. Tomohiro SHIRAKI, Akiko Tsuzuki, Fumiyuki TOSHIMITSU, Naotoshi NAKASHIMA, Thermodynamics for the Formation of Double-stranded DNA-Single-walled Carbon Nanotube Hybrids, Chemistry - A European Journal, 10.1002/chem.201504533, 22, 4774-4779, Selected as very important paper (VIP) and inside cover, 2016.01.
14. Tomonari Shiraishi, JUHASZ GERGELY MIKLOS, Tomohiro SHIRAKI, Naoto Akizuki, Yuhei Miyauchi, Kazunari Matsuda, Naotoshi NAKASHIMA, Determination of Precise Redox Properties of Oxygen-Doped Single-Walled Carbon Nanotubes Based on in Situ Photoluminescence Electrochemistry, The Journal of Physical Chemistry C, 10.1021/acs.jpcc.5b07841, 120, 15632-15639, 2015.11.
15. Tomohiro SHIRAKI, Gayoung KIM, Naotoshi NAKASHIMA, Room Temperature Synthesis of a Covalent Organic Framework with Enhanced Surface Area and Thermal Stability and Application to Nitrogen-doped Graphite Synthesis, Chemistry Letters, 44, 1488-1490, 2015.11.
16. Xiaojing Yu, Tomohiro SHIRAKI, Shengchun Yang, Bingjun Dinga, Naotoshi NAKASHIMA, Synthesis of porous gold nanoparticles/MoS2 nanocomposites based on redox reaction, RSC Advances, 10.1039/C5RA15421A , 5, 86558-86563, 2015.09.
17. Tomohiro SHIRAKI, Shoichiro SHINDOME, Fumiyuki TOSHIMITSU, Tsuyohiko FUJIGAYA, Naotoshi NAKASHIMA, Strong Main-Chain Length-Dependence for the ß-Phase Formation of Oligofluorenes , Polymer Chemistry, 10.1039/C5PY00385G , 6, 5103-5109, 2015.06.
18. Tomohiro SHIRAKI, Naotoshi NAKASHIMA, In Situ Photoluminescence Spectroelectrochemistry for Determination of Electronic States of Single-walled Carbon Nanotubes, e-Journal of Surface Science and Nanotechnology, 10.1380/ejssnt.2015.179, 13, 179-184, 2015.04.
19. JongTae Yoo, SuHyun Lee, Shinsuke Hirata, ChaeRin Kim, Chang Kee Lee, Tomohiro SHIRAKI, Naotoshi NAKASHIMA, Jin Kie Shim, In Situ Synthesis of Covalent Organic Frameworks (COFs) on Carbon Nanotubes and Graphenes by Sonochemical Reaction for CO2 Adsorbents, Chemistry Letters, 10.1246/cl.141194, 44, 4, 560-562, 2015.04.
20. Jun Li, Tomohiro Shiraki, Bin Hu, Roger A. E. Wright, Bin Zhao, Jeffrey S. Moore, Mechanophore Activation at Heterointerfaces, Journal of the American Chemical Society, 136, 15925-15928, 2014.10.
21. Tomohiro Shiraki, Charles E. Diesendruck, Jeffrey S. Moore, Mechanochemical production of phenyl cations through heterolytic bond scission, Faraday Discussions, 170, 385-394, 2014.12.
Presentations
1. Tomohiro Shiraki, Yoshiaki Niidome, Fumiyuki Toshimitsu, Tsuyohiko Fujigaya, Microenvironment Effects on Photoluminescent Doped Sites of Locally Functionalized Single-walled Carbon Nanotubes, 235th ECS Meeting, 2019.05.
2. Tomohiro Shiraki, Tamehito Shiga, Naotoshi Nakashima, Tsuyohiko Fujigaya, Post-Chemical Modification of Doped Sites of Locally Functionalized Single-Walled Carbon Nanotubes for Multistep Photoluminescence Modulation, 235th ECS Meeting, 2019.05.
3. Tomohiro Shiraki, Molecularly-modulated Energy of Exciton Confined in the One Dimensional Nanostructures of Single-walled Carbon Nanotubes, 2019 MRS Spring Meeting & Exhibit, 2019.04.
4. Tomohiro Shiraki, Hisashi Onitsuka, Tamehito Shiga,Tomonari Shiraishi, Naotoshi Nakashima, Tsuyohiko Fujigaya, Selective Wavelength Shifts of Near Infrared Photoluminescence Based on Molecular Recognition on Single-walled Carbon Nanotubes, 12th SPSJ International Polymer Conference (IPC2018), 2018.12.
5. Tomohiro Shiraki, Near Infrared Photoluminescence Tuning Driven by Molecular Recognition on Single-walled Carbon Nanotubes, MIRAI Workshop - Materials Science, 2018.10.
6. Tomohiro Shiraki, Near infrared photoluminescent nanomaterials whose functions are tunable based on molecular interactions, 第67回高分子討論会 日韓ジョイントセッション/Japan-Korea Joint Session, 2018.09.
7. Tomohiro Shiraki, Molecular design for photoluminescence modulation of locally functionalized single-walled carbon nanotubes, 7th Workshop on Nanotube Optics and Nanospectroscopy (WONTON 2018), 2018.07, 開発を行っている高効率な近赤外発光を示す局所化学修飾単層カーボンナノチューブにおいて、修飾サイトの分子構造デザインという独自の戦略から様々な物性や機能を開拓した。.
8. Tomohiro Shiraki, Shunsuke Uchimura, Tomonari Shiraishi, Fumiyuki Toshimitsu, Naotoshi Nakashima, Substituted Aryl Structure Effects on Photoluminescence Properties of Locally Functionalized Single-Walled Carbon Nanotubes, 233rd ECS Meeting, 2018.05, 開発を行っている高効率な近赤外発光を示す局所化学修飾単層カーボンナノチューブにおいて、修飾分子の異性体構造に基づく分子構造変化に応じた顕著な発光特性を導くことに成功した研究.
9. Tomohiro Shiraki, Hisashi Onitsuka, Tamehito Shiga, Naotoshi Nakashima, Molecular Recognition at Local Doped Sites of Locally Functionalized Single-Walled Carbon Nanotubes for Selective Wavelength Shift of Near Infrared Photoluminescence, 233rd ECS Meeting, 2018.05.
10. Tomonari Shiraishi, Tomohiro SHIRAKI, Naotoshi NAKASHIMA, Proximal Modification for Near Infrared Photoluminescence Modulation of Carbon Nanotubes, 2017 MRS FALL MEETING & EXHIBIT, 2017.11.
11. Tamehito SHIGA, Naotoshi NAKASHIMA, Tomohiro SHIRAKI, Near Infrared Emission Wavelength Modulation Based on Post-Modification Using Imine Bond Formation on Single-Walled Carbon Nanotubes, 2017 MRS FALL MEETING & EXHIBIT, 2017.11.
12. Tomohiro SHIRAKI, Gayoung Kim, Jung Yang, Naotoshi NAKASHIMA, Microporous Nitrogen-Doped Carbon Synthesis through Direct Carbonization of Covalent Organic Frameworks, 2017 MRS FALL MEETING & EXHIBIT, 2017.11.
13. Tomohiro SHIRAKI, Tomonari SHIRAISHI, Hisashi ONITSUKA, Tamehito SHIGA, Gergely Juhász, Naotoshi NAKASHIMA, Molecularly-Functionalized Near Infrared Photoluminescence Properties of Single-Walled Carbon Nanotubes, 2017 MRS FALL MEETING & EXHIBIT, 2017.11.
14. Tomohiro Shiraki, Surface Functionalization of Single-Walled Carbon Nanotubes towards Novel Near-Infrared Photoluminescent Materials, MIRAI Workshop - Materials Science, 2017.10.
15. Tomohiro SHIRAKI, Tomonari SHIRAISHI, Hisashi ONITSUKA, Tamehito SHIGA, Gergely Juhász, Naotoshi NAKASHIMA, Chemistry-based functionalization of single-walled carbon nanotubes toward their photoluminescence property modulation, 第53回 フラーレン・ナノチューブ・グラフェン総合シンポジウム, 2017.09.
16. Tomohiro Shiraki, Hisashi Onitsuka, Tomonari Shiraishi, Naotoshi Nakashima, Photoluminescent Readout of Molecular Information Using Local Sites Functionalized on Single-Walled Carbon Nanotubes, 231st ECS Meeting, 2017.05.
17. Tomohiro Shiraki, Tomonari Shiraishi, Hisashi Onitsuka, Gergely Juhász, Naotoshi Nakashima, Effects of Chemically-Introduced Structures on Near Infrared Photoluminescence of Locally Functionalized
Single-Walled Carbon Nanotubes, 231st ECS Meeting, 2017.05.
18. Tomohiro Shiraki, Tomonari Shiraishi, Hisashi Onitsuka, Gergely Juhász, Naotoshi Nakashima, Near-Infrared Photoluminescence Modulation of Carbon Nanotubes Based on Molecular Design of Chemical Modification Sites, The 11th SPSJ International Polymer Conference (IPC2016), 2016.12.
19. Tomonari Shiraishi, Tomohiro Shiraki, Naotoshi Nakashima, Emergence of a New Near-IR Photoluminescence of Carbon Nanotubes by Adjacent Chemical Modification, The 11th SPSJ International Polymer Conference (IPC2016), 2016.12.
20. Gayoung Kim, Tomohiro Shiraki, Naotoshi Nakashima, Nitrogen-doped carbon materials with high porosity synthesized from covalent organic frameworks, The 11th SPSJ International Polymer Conference (IPC2016), 2016.12.
21. Hisashi Onitsuka, Tomohiro Shiraki, Naotoshi Nakashima, Photoluminescence spectral shift induced by sugar recognition on phenyl boronic acid-modified single-walled carbon nanotubes, The 11th SPSJ International Polymer Conference (IPC2016), 2016.12.
22. Koichiro Uchida, Tomohiro Shiraki, Naotoshi Nakashima, Photoluminescence of carbon dots using energy transfer systems, The 11th SPSJ International Polymer Conference (IPC2016), 2016.12.
23. Gayoung Kim, Tomohiro Shiraki, Naotoshi Nakashima, Fabrication of Nitrogen-Doped Porous Carbon from Covalent Organic Frameworks and the Electrocatalytic Activities for Oxygen Reduction Reaction, PRiME 2016/230th ECS Meeting, 2016.10.
24. Tomohiro Shiraki, Tomonari Shiraishi, Hisashi Onitsuka, Naotoshi Nakashima, Photoluminescence modulation of single-walled carbon nanotubes based on local-covalent modification using designed molecules, Seventeenth International Conference on the Science and Application of Nanotubes and low-dimensional materials (NT16), 2016.08.
25. Tomohiro Shiraki, Gayoung KIM, 中嶋 直敏, Covalent Organic Frameworks Carbonized for Synthesis of Functional Carbon Materials, 第65回高分子学会年次大会 高分子学会, 2016.05.
26. Gayoung Kim, Tomohiro Shiraki, Naotoshi Nakashima, A two-dimensional organic layered material with high crystallinity by a room temperature synthesis, 6th A3 Symposium on Emerging Materials, 2015.11.
Membership in Academic Society
  • The Society of Polymer Science, Japan (SPSJ)
  • The Chemical Society of Japan (CSJ)
  • The Fullerenes, Nanotubes and Graphene Research Society (FNTG)
Educational
Educational Activities
Guidance of experimental class (Undergraduate, 3rd year)
Guidance of experimental class (Undergraduate(G30), 3rd year)
Analytical Chemistry practice class (Undergraduate, 3rd year)
Research guidance in the lab (Undergraduate, 4th year)
Research guidance in the lab (Master, Doctor course)
Social
Professional and Outreach Activities
Open campus for high school students etc.
Arrangement for visitors including domestic and foreign researchers and scientific discussions.